Quantum criticality in an organic magnet
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Exchange interactions between S=½ sites in piperazinium hexachlorodicuprate produce a frustrated bilayer magnet with a singlet ground state. We have determined the field-temperature phase diagram by high field magnetization and neutron scattering experiments. There are two quantum critical points: Hc1=7.5 T separates a quantum paramagnet phase from a three dimensional, antiferromagnetically ordered state while Hc2=37 T marks the onset of a fully polarized state. The ordered phase, which we describe as a magnon Bose-Einstein condensate (BEC), is embedded in a quantum critical regime with short range correlations. A low temperature anomaly in the BEC phase boundary indicates that additional low energy features of the material become important near Hc1.
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Diallo, S.O.; Antropov, V.P.; Perring, T.G.; Broholm, C.; Pulikkotil, J.J.; Ni, N.; Bud'ko, S.L.; Canfield, P.C.; Kreyssig, A.; Goldman, A.I.; McQueeney, R.J. (American Physical Society, 2009-05-08)Neutron scattering measurements of the magnetic excitations in single crystals of antiferromagnetic CaFe2As2 reveal steeply dispersive and well-defined spin waves up to an energy of ~100 meV. Magnetic excitations above 100 ...
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